Bridging interfacial water structure and reactivity in photocatalytic hydrogen evolution at TiO₂ interfaces
Hydrogen (H2) evolution via photocatalytic water splitting is an environmentally friendly and sustainable technology for solar-to-chemical energy conversion. Although interfacial interactions are recognized as key determinants of photocatalytic performance, systematic experimental studies explicitly targeting the structure and reactivity of the water-catalyst interface remain limited. A major challenge lies in probing the molecular structure of interfacial water, especially under hydrogen-evolving conditions.
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